Transition Metal Catalysis in Macromolecular Design

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Metal-mediated polymerization is fast becoming an essential tool for the fine control of macromolecular architecture. Advanced Catalysis demonstrates how the field of transition metal-catalyzed polymer syntheses has moved beyond the simple use of single-site catalysts to new applications and "advanced" techniques of architectural control. This book defines and presents "next generation" techniques and trends for polymer architecture control for an immediate grasp on the future ...
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Overview


Metal-mediated polymerization is fast becoming an essential tool for the fine control of macromolecular architecture. Advanced Catalysis demonstrates how the field of transition metal-catalyzed polymer syntheses has moved beyond the simple use of single-site catalysts to new applications and "advanced" techniques of architectural control. This book defines and presents "next generation" techniques and trends for polymer architecture control for an immediate grasp on the future of this exciting field.
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Product Details

  • ISBN-13: 9780841236738
  • Publisher: American Chemical Society
  • Publication date: 7/20/2000
  • Series: ACS Symposium Series , #760
  • Pages: 312
  • Product dimensions: 6.10 (w) x 9.10 (h) x 0.80 (d)

Meet the Author

Exxon Research & Engineering Company

North Carolina State University

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Table of Contents

Preface ix
1. The Organometallic Polymerization of (Meth)acrylates: An Overview 1
New Chain-Building Mechanisms
2. New Applications of "Carbonylbis(triphenylphosphine)ruthenium" Catalysis in Polymer Synthesis 24
3. Transition Metal-Catalyzed Alkyne Cycloaddition Polymerization 38
4. Synthetic Control over Substituent Location on Carbon-Chain Polymers Using Ring-Opening Polymerization of Small Cycloalkanes 59
5. Nucleophilic Polymerization of Methyl Methacrylate Activated by a Bronsted Acid 77
Polymer Modification Using Transition Metals
6. Modification of Polybutadiene by Transition Metal Catalysts: Hydroacylation of Polybutadiene 94
7. Metallocene Catalysts Used for the Hydrogenation of Polystyrene-b-Polybutadiene-b-Polystyrene Block Copolymers 108
8. E-Glass Fiber Supported Hydrosilation Catalysts 127
Olefin/Alkyne Addition Polymerization
9. New Catalysts for Polymerizations of Substituted Acetylenes 146
10. Addition Polymerization of Norbornene: Catalysis of Monocyclopentadienyltitanium Compounds Activated with Methylaluminoxane 165
11. Transfer and Isomerization Reactions in Propylene Polymerization with the Isospecific, Highly Regiospecific rac-Me[subscript 2]C(3-t-Bu-1-Ind)[subscript 2]ZrCl[subscript 2]/MAO Catalyst 174
Controlled Radical Polymerization
12. Living Radical Polymerization of Acrylates with Rhenium(V)-Based Initiating Systems: ReO[subscript 2]I(PPh[subscript 3])[subscript 2]/Alkyl Iodide 196
13. The Effect of Ligands on Copper-Mediated Atom Transfer Radical Polymerization 207
14. Structural Chemistry and Polymerization Activity of Copper(I) Atom Transfer Radical Polymerization Catalysts 224
15. Atom Transfer Polymerization Mediated by Solid-Supported Catalysts 236
16. Mechanistic Aspects of Catalytic Chain Transfer Polymerization 254
Indexes
Author Index 275
Subject Index 276
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