Measuring Fundamental Symmetry Violation in Polyatomic Molecules

This thesis presents major advances toward the realization of quantum control in complex molecules for applications in precision metrology. Polyatomic molecules engineered to be sensitive to new fundamental particles and forces are a powerful platform to search for physics beyond the Standard Model. A major limitation to this application, as well as any other relying on the complete quantum control of complex polyatomic molecules, is that fully understanding them remains a research frontier...